"Bad Guy" is a very vague term and there are several villains in the Smurfs series. Here are some of the major villains:
Gargamel - He is the main antagonist of the Smurfs. He is an evil wizard who wants to capture the Smurfs and use them for his experiments. His main goal is to turn the Smurfs into gold.
Azrael - Gargamel's pet cat who helps him in his plans to catch the Smurfs.
Scruple - Gargamel's apprentice who is always trying to earn his master's approval by helping him catch the Smurfs.
Lord Balthazar - He is a villain from the Smurfs movie. He wants to capture Smurfette and use her to turn his grey army into blue ones.
Viviane - She is a villain from the Smurfs comics. She is a female wizard who tries to seduce Papa Smurf and use him for her own selfish purposes.
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